Hi there and welcome.
I'm not too familiar with the MT4x (used them a LONG time ago!), but the principle is still the same:
Firstly, stripe a track (conventionally track 4) with timecode/LTC*. (Unitor LTC
out to MTX4x input 4.)
You will need a SMPTE convertor/generator: something like Unitor 8 mk2 is probably the most obvious (assuming you're using Mac).
Secondly, plug mt4x output/track 4 BACK
in to LTC in on the Unitor 8.
This will enable the Unitor to "hear" the LTC/SMPTE track.
In Logic, all you do is enable 'auto sync in" (IIRC! It's 7.20am here, writing this in bed with a cuppa!).
There are some caveats to this though -
*SMPTE/LTC operates in the following format:-
00:00:00:00.00 (hours:minutes:seconds:frames.subframes)
When using this with tape, I would always stripe the ENTIRE tape from 01 hours. Then each consecutive tape would be striped from the next hour (easy way of "labelling" tapes - BUT tends to work timescale-wise (!) on open-reel tape!)
I always striped from zero, but would put a SMPTE start-time in Logic/DAW of 30 seconds.
You ALSO
MUST make sure that what ever you record on track 3, is relatively quiet, as tape suffers from bleed-through (where consecutive track audio can be "heard" on the adjacent tracks.
Therefore, imho and experience, the SMPTE track must be protected, as it is a TOTAL PAIN IN THE A$$ to repair a timecode track.
That said, if you're using Logic, why bother with the MT4x?
1. You'll only gain 2 tracks of "analogue" recording with a 3rd track to be VERY careful with.
2. If it's for stuff you've already got on 4-track, just record it into Logic - even if your machine only has a stereo out: record the tracks over 2 passes (2 tracks at a time) - you can then move them back in sync (bit of a bodge, but it works)
Hope this helps - if you're not used to dealing with syncing, it's a bit of a daunting prospect, but again:-
**Stripe (record SMPTE/LTC) your tape FIRST!**
This will overcome MOST of your potential problems, and will make the process easier!
All the best,
Dan (remembering his SMPTE nightmares!!

)
ps you can use other SMPTE/LTC stripe/read boxes, but you'd have to do some more RTFM!!